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Research in Professor Morse’s group is directed toward understanding the chemical bonding and electronic structure in metallic and semiconductor systems by detailed spectroscopic investigations. This research makes extensive use of laser spectroscopy through laser-induced fluorescence, resonant two-photon ionization, and photodissociation action spectroscopy of mass-selected cations. In many of these experiments, metal or semiconductor atoms are ablated from an appropriate target in the throat of a pulsed supersonic expansion by a focused laser pulse. Condensation of the atomic species then occurs in the high pressure region downstream from the point of vaporization. Expansion into vacuum cools the molecules to a few degrees Kelvin, then isolates them from further collisions as the pressure drops. Farther downstream, a variety of spectroscopic experiments are performed, aimed at understanding the molecular structure (both electronic and geometrical) of the small metal and semiconductor molecules.
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The Journal of chemical physicsno. 8 (2024)
INORGANIC CHEMISTRYno. 24 (2023): 9589-9601
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Dakota M Merriles, Annie S Knapp, Yexalen Barrera-Casas,Andrew Sevy,Jason J Sorensen,Michael D Morse
JOURNAL OF CHEMICAL PHYSICSno. 7 (2022): 074303
Proceedings of the 2021 International Symposium on Molecular Spectroscopy (2021)
Proceedings of the 2021 International Symposium on Molecular Spectroscopy (2021)
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