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个人简介
Professor Scheidt obtained his Ph.D. in inorganic chemistry at the University of Michigan. After postdoctoral work at Cornell University, where he became interested in the chemistry and stereochemistry of metalloporphyrin complexes, he joined the faculty of the University of Notre Dame, where he is now Warren Professor. He has been a visiting professor at the University of Washington, University of Paris(Orsay and Rene Decartes) and University Louis Pasteur (Strasbourg, France). In addition to more than 250 scientific publications, he has authored several book chapters. He is an elected fellow of the American Association for the Advancement of Science.
Research Interests:
In all of our studies, we work on the preparation of new metalloporphyrin compounds, especially biologically important iron, that allow us to explore their properties using a number of techniques. These include methods that allow us to to investigate electronic structure (Elelctron Paramagnetic Resonance and Mössbauer spectroscopy, magnetic susceptibilities, and calculations), molecular structure (X-ray and neutron diffraction), and electronic and vibrational spectroscopy (especially NRVS, IR and Raman).
Recent Papers:
Silvernail, N. J.; Pavlik, J. W.; Noll B. C.; Schulz, C. E.; Scheidt, W. R. Reversible NO Motion in Crystalline [Fe(Porph)(1-MeIm)(NO)] Derivatives. Inorg. Chem. 2008, 47, 912– 920
。 Hu, C.; Roth, A.; Ellison, M. K.; An, J.; Ellis, C. M.; Schulz, C. E.; Scheidt, W. R. Electronic Configuration Assignment and the Importance of Low-Lying Excited States in High-Spin Imidazole-Ligated Iron(II) Porphyrinates. J. Am. Chem. Soc. 2005, 127, 5675–5688.
Leu, B. M.; Silvernail, N. J.; Zgierski, M. Z.; Wyllie, G. R. A.; Ellison, M. K.; Scheidt, W. R.; Zhao, J.; Sturhahn, W.; Alp, E. E.; Durbin, S. M.; Sage, J. T. Quantitative Vibrational Dynamics of Iron in Carbonyl Porphyrins. Biophys. J. 2007, 92, 3764–3783.
Li, J.; Lord, R. L.; Noll, B. C.; Baik, M.-H.; Schulz, C. E.; Scheidt, W. R. Cyanide: a Strong Field Ligand for Ferrohemes and Hemoproteins? Angew. Chem., Int. Ed., 2008, 47, 10144–10146. (recognized with the cover)
。Silvernail, N. J.; Barabanschikov, A.; Sage, J. T.; Noll, B. C.; Scheidt, W. R. Mapping NO Movements in Crystalline [Fe(Porph)(NO)(1-MeIm)]. J. Am. Chem. Soc. 2009, 131, 2131–2140.
。 Hu, C.; Noll, B. C.; Piccoli, P. M. B.; Schultz, A. J.; Schulz, C. E.; Scheidt, W. R. Hy- drogen Bonding Effects on the Electronic Conguration of Five-Coordinate High-Spin Iron(I I) Porphyrinates. J. Am. Chem. Soc. 2008, 130, 3127–3136.
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