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Control Of Chemical Reactions By Feedback-Optimized Phase-Shaped Femtosecond Laser Pulses

SCIENCE, no. 5390 (1998): 919-922

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Tailored femtosecond laser pulses from a computer-controlled pulse shaper were used to optimize the branching ratios of different organometallic photodissociation reaction channels. The optimization procedure is based on the feedback from reaction product quantities in a Learning evolutionary algorithm that iteratively improves the phase ...更多

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