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Decoherence Of Excitons In Multichromophore Systems: Thermal Line Broadening And Destruction Of Superradiant Emission

PHYSICAL REVIEW LETTERS, no. 17 (2005)

Cited: 95|Views22

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Abstract

We study the temperature-dependent dephasing rate of excitons in chains of chromophores, accounting for scattering on static disorder as well as acoustic phonons in the host matrix. From this we find a power-law temperature dependence of the absorption linewidth, in excellent quantitative agreement with experiments on dye aggregates. We a...More

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D. J. Heijs

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V. A. Malyshev

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J. Knoester

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