Direct Measurement Of Giant Electrocaloric Effect In Batio3 Multilayer Thick Film Structure Beyond Theoretical Prediction

APPLIED PHYSICS LETTERS(2010)

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摘要
The electrocaloric (EC) effect of BaTiO3 multilayer thick film structure was investigated by direct measurement and theoretical calculation. The samples were prepared by the tape-casting method, which had 180 dielectric layers with an average thickness of 1.4 mu m. The thermodynamic calculation based on the polarization-temperature curves predicted a peak heat adsorption of 0.32 J/g at 80 degrees C under 176 kV/cm electric field. The direct measurement via differential scanning calorimeter showed a much higher EC effect of 0.91 J/g at 80 degrees C under same electric field. The difference could result from the different trends of changes of electric polarization and lattice elastic energy under ultrahigh electric field. (C) 2010 American Institute of Physics. [doi:10.1063/1.3430045]
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关键词
barium compounds, dielectric polarisation, differential scanning calorimetry, ferroelectric ceramics, lattice energy, multilayers, pyroelectricity, tape casting, thermodynamic properties
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