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Two-Pulse Field-Free Orientation Reveals Anisotropy Of Molecular Shape Resonance

PHYSICAL REVIEW LETTERS, no. 2 (2014): 023001-023001

Cited: 85|Views19

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pubmed.ncbi.nlm.nih.gov academic.microsoft.com arxiv.org

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We report the observation of macroscopic field-free orientation, i.e., more than 73% of CO molecules pointing in the same direction. This is achieved through an all-optical scheme operating at high particle densities(> 10(17) cm(-3)) that combines one-color (omega) and two-color (omega + 2 omega) nonresonant femtosecond laser pulses. We s...More

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P M Kraus

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D Baykusheva

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H J Wörner

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