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Two-Pulse Field-Free Orientation Reveals Anisotropy Of Molecular Shape Resonance
PHYSICAL REVIEW LETTERS, no. 2 (2014): 023001-023001
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Abstract
We report the observation of macroscopic field-free orientation, i.e., more than 73% of CO molecules pointing in the same direction. This is achieved through an all-optical scheme operating at high particle densities(> 10(17) cm(-3)) that combines one-color (omega) and two-color (omega + 2 omega) nonresonant femtosecond laser pulses. We s...More
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