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Radical Philicity Inversion in Co- and Fe-Catalyzed Hydrogen-Atom-Transfer-Initiated Cyclizations of Unsaturated Acylsilanes

ACS Catalysis, no. 1 (2020): 510-515

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Abstract

[1,2]-Radical Brook rearrangement (RBR) has been identified as a viable pathway in M–H (M = Co, Fe) catalyzed hydrogen-atom-transfer reactions involving unsaturated acylsilanes. Guided by the same concept, we have explored two transformations, namely, a Co-catalyzed cycloisomerization reaction and a Fe-catalyzed cyclization/Giese addition...More

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