International cooperation in age-dating uranium standards for nuclear forensics using the 231 Pa/ 235 U radiochronometer

Journal of Radioanalytical and Nuclear Chemistry(2020)

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摘要
During 2017–2018 Los Alamos National Laboratory, Lawrence Livermore National Laboratory and the China Institute of Atomic Energy collaborated in an interlaboratory 231 Pa/ 235 U radiochronometry exercise. The laboratories used different analytical methods to obtain a consensus model purification date for CRM U010 of December 28, 1958 ± 198 days and for CRM U850 of May 20, 1958 ± 363 days. These results agree with previously reported model dates using the 230 Th/ 234 U radiochronometer as well as the production histories of these materials. The concordance of interlaboratory data confirms the ability of laboratories to make reproducible radiochronometry measurements using distinct analytical approaches.
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关键词
Radiochronometry, Protactinium, Certified reference material, Nuclear forensics, Uranium
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