Stable metal-organic frameworks with low water affinity built from methyl-siloxane linkers.

Luke C Delmas,Andrew J P White,David Pugh,Arwyn Evans, Mark Antonin Isbell,Jerry Y Y Heng,Paul D Lickiss,Robert P Davies

CHEMICAL COMMUNICATIONS（2020）

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摘要

A tetracarboxylic acid with a methyl-substituted siloxane core (L-H-4) has been prepared and applied in the construction of water stable MOFs with low water affinity.L-H(4)itself crystallizes as an interpenetrated 3D hydrogen-bonded network. Reaction ofL-H(4)with Zr-IV/Hf(IV)gave IMP-32-Zr/Hf - both 3D MOFs ofscutopology.

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