Encapsulated X-Ray Detector Enabled by All-Inorganic Lead-Free Perovskite Film With High Sensitivity and Low Detection Limit
IEEE Transactions on Electron Devices(2020)
摘要
The sensitive detection of low-dose X-ray radiation is essential to many X-ray applications. In this article, the ultrasensitive X-ray detector based on pure Cs
2
AgBiBr
6
all-inorganic lead-free perovskite film is successfully demonstrated and encapsulated using a metal casing with a Be window. The high-quality Cs
2
AgBiBr
6
films are obtained through the low-cost solution process with long electron–hole diffusion length (~700 nm) and long carrier lifetime (~750 ns). Benefiting from the excellent properties of the Cs
2
AgBiBr
6
film and the stable ambient provided by the packaging module, the resulting device exhibits attractive X-ray detection capabilities with a minimum detectable dose rate of 145.2
${\mathrm {nGy}}_{air}\text{s}^{-1}$
and a detection sensitivity up to
$1.8\times 10^{4}\,\,\mu {\mathrm {CGy}}_{air}{}^{-1}$
cm
−2
, which is about a thousand times higher than the sensitivity achieved with commercial a-Se X-ray detectors. Besides, the encapsulated device maintains superior detection performance after 2 months of storage, indicating the favorable reliability of the encapsulated device. This article demonstrates a possibility to use Cs
2
AgBiBr
6
perovskite film and Be window for the sensitive X-ray detection, which will inspire further development of radiation electronics by utilizing all-inorganic lead-free perovskite.
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关键词
Lead,Detectors,X-ray detectors,Sensitivity,Crystals,X-ray detection,Encapsulation
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