Analysis of spatiotemporal variation of formaldehyde column concentration in Qinghai-Tibet Plateau and its influencing factors

ENVIRONMENTAL SCIENCE AND POLLUTION RESEARCH(2021)

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摘要
Based on the formaldehyde (HCHO) inversion data of OMI satellite sensor from 2009 to 2019, this paper discusses the spatial and temporal distribution of HCHO column concentration over the Qinghai-Tibet Plateau in the past 11 years and explores the factors affecting the dynamic distribution of atmospheric HCHO column concentration over the Qinghai-Tibet Plateau in combination with meteorological, aerosol, ozone, and other data. The results show that the average concentration of HCHO column in the Qinghai-Tibet Plateau is 8.84 × 10 15 molec/cm 2 in the past 11 years, which is relatively low, and the annual variation rate of HCHO column is 7.79%, showing a slight upward trend. The seasonal changes show a trend of Autumn < Winter < Spring < Summer. The monthly variation is more obvious than the seasonal variation. The spatial distribution showed a decreasing trend from southeast to northwest. Residual analysis showed that 83.77% of the area was frequently affected by natural factors. Correlation analysis found that the natural factors including precipitation, air temperature, and atmospheric activities for a greater influence on the column experiment the distribution of the concentration of the Qinghai-Tibet Plateau and human factors, such as biomass, the distribution of fossil fuel combustion, and emissions to HCHO, play a promoting role. Through the backward trajectory analysis, it can be seen that the transboundary atmospheric transport activity has a prominent contribution to the distribution of HCHO in the southern region of the Qinghai-Tibet Plateau. Hurst index study found that in the future, the concentration of HCHO column in 53.03% of the Qinghai-Tibet Plateau will decrease, but in some areas, such as the eastern and northern parts of the Qinghai-Tibet Plateau, it will increase.
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关键词
Qinghai-Tibet Plateau, OMI, HCHO column concentration, Backward trajectory, Influencing factors
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