Atomic-level active sites of efficient imidazolate framework-derived nickel catalysts for CO₂ reduction

Fuping Pan,Hanguang Zhang,Zhenyu Liu,David Cullen,Kexi Liu,Karren More,Gang Wu,Guofeng Wang,Ying Li

Journal of Materials Chemistry A（2019）

引用 56|浏览3

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摘要

Active sites of single-atom nickel catalysts for CO2 reduction were revealed to be edge-located Ni–N2+2 sites with dangling bond-containing carbon atoms, which facilitate the dissociation of the C–O bond of *COOH intermediate.

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Atomic-level active sites of efficient imidazolate framework-derived nickel catalysts for CO2 reduction

Atomic-level active sites of efficient imidazolate framework-derived nickel catalysts for CO₂ reduction