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Spin to charge conversion in chemically deposited epitaxial La0.9MnO3 thin films capped with Pt

Journal of materials chemistry C(2022)

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摘要
Spin to charge conversion process in a broad range of temperatures is studied in La0.92MnO3/Pt bilayers prepared by polymer-assisted deposition (PAD). It is shown that an excellent LMO/Pt interface can be obtained in spite of using ex situ deposition of the Pt layer. The values obtained for the effective spin-mixing conductance, g up arrow down arrow(eff) = 0.76 x 10(15) cm(-2), suggest that significant spin transport across the LMO/Pt interface could be achieved. Spin pumping experiments generate a transversal voltage signal V-ISHE, due to spin to charge conversion via inverse spin Hall effect, that has been detected down to about 100 K with values of the spin-Hall angle, theta(SH), of about 2.5%, slightly decreasing on reducing temperature in the analyzed temperature range. These results indicate that LMO is a promising perovskite building block for all-oxide multifunctional high-frequency spintronics devices and that PAD technique provides oxide epitaxial thin films of good quality adequate for spintronic applications.
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