Evaluation of the simulated aerosol optical properties over India: COALESCE model inter-comparison of three GCMs with ground and satellite observations.

Within the framework of COALESCE project (Carbonaceous aerosol emissions, source apportionment, and climate impacts) initiative, spatio-temporal distribution of aerosol optical properties from three general circulation models are evaluated against aerosol data from satellite observations (MODIS and CALIPSO) and ground-based measurements (AERONET) for the period 2005-2014. The GCMs, NICAM-SPRINTARS (N-S), ECHAM6.3-HAM2.3 (E-H), CAM5.3 (CAM), input with identical emissions from the SMoG-India-v1 emission inventory over India nested in the CEDS global inventory, including all emission sectors except sea salt and soil dust. The annual mean total aerosol optical depth (AOD) averaged over the Indian land region is 0.38, 0.27, and 0.17 from the N-S, CAM, and E-H models respectively, while the annual mean value from the MODIS observational dataset is 0.43. Single scattering albedo predicted by E-H is lower compared to CAM and N-S while model predictions of Angstrom exponent are closer to MERRA2 dataset. However, the average total aerosol column burden over Indian landmass simulated by the models is very close and comparable to the reanalysis results. Statistical analysis of AOD between model and AERONET measurements at nine sites shows that the root mean square error varies from 0.1 to 0.4 and the index of agreement (average value) is ∼0.4. The aerosol emission and transport models, methodology for calculation of aerosol optical properties and their mixing states contributes to the diversity in the results from various models. The present study provides an analysis of limitations and uncertainties contributing to the differences between the simulations and observations, and the inter-model diversity.