Magnetic domain depinning as possible evidence for two ferromagnetic phases in LaCrGe3

Two ferromagnetic phases, FM1 and FM2, were first proposed to exist in LaCrGe3 based on a broad maximum in the temperature derivative of resistivity resembling that of the superconducting ferromagnet UGe2 where FM1 and FM2 are well-established. While evidence for two FM phases can be found in certain additional probes, corresponding anomalies in magnetization have not been recognized until now. Our spatially resolved images of the magnetic domains show a substantial change in the domain structure between the higher temperature FM1 phase and the lower temperature FM2 phase. Furthermore, our measurements of the coercive field and virgin magnetization curves reveal an unconventional magnetic domain pinning region in the FM1 phase, followed by a depinning region at lower temperatures where the system is reported to crossover into the FM2 phase. We incorporate this discovery into a simple domain magnetization model that demystifies the magnetization curve seen in all previous studies. Finally, we find that the unusual domain behavior can be explained by a change in the magnetic moment and the presence of two ferromagnetic exchange constants, both of which are consistent with the existence of two FM phases. This revelation may help explain a range of anomalous behaviors observed in LaCrGe3 and rekindles the discussion about the prevalence of multiple FM phases in fragile FM systems.