From Cs8Sb4Nb5O5F35 to Cs6Sb4Mo3O5F26: The first noncentrosymmetric fluoroantimonite with d0 transition metal

Jia-Hang Wu,Bo Zhang,Ting-Kun Jiang,Fang Kong,Jiang-Gao Mao

Chinese Journal of Structural Chemistry（2023）

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摘要

The first noncentrosymmetric d0 TM fluoroantimonate, Cs6Sb4Mo3O5F26, has been achieved by substituting the d0 TM in centrosymmetric Cs8Sb4Nb5O5F35. Cs6Sb4Mo3O5F26 features a phase-matchable SHG response of about 72% of the commercial KDP. Its powder laser-induced damage threshold (133.5 MW/cm2) is about 33.4 times that of AGS (4.0 MW/cm2).Image 1

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first noncentrosymmetric fluoroantimonite,transition metal,cs6sb4mo3o5f26,cs8sb4nb5o5f35

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