Mixed 3D-2D Perovskite Flexible Films for the Direct Detection of 5 MeV Protons

ADVANCED SCIENCE(2023)

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摘要
This study reports on a novel, flexible, proton beam detector based on mixed 3D-2D perovskite films deposited by solution onto thin plastic foils. The 3D-2D mixture allows to obtain micrometer-thick and highly uniform films that constitute the detector's active layer. The devices demonstrate excellent flexibility with stable electric transport properties down to a bending radius of 3.1 mm. The detector is characterized under a 5 MeV proton beam with fluxes in the range [4.5 x 10(5) - 1.4 x 10(9)] H+ cm(-2) s(-1), exhibiting a stable response to repetitive irradiation cycles with sensitivity up to (290 +/- 40) nC Gy(-1)mm(-3) and a limit of detection down to (72 +/- 2) mu Gy s(-1). The detector radiation tolerance is also assessed up to a total of 1.7 x 10(12) protons impinging on the beam spot area, with a maximum variation of the detector's response of 14%.
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关键词
2D-3D perovskites, dosimetry, flexible radiation detectors, perovskites, proton detectors, thin films
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