A promising (Yb0.2Tm0.2Lu0.2Sc0.2Er0.2)2Si2O7 with excellent thermophysical properties for thermal environmental barrier coatings material

Journal of Alloys and Compounds(2024)

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摘要
Aiming at the development of thermal environmental barrier coatings (TEBCs) material, the factor of grain size is introduced into the high-entropy rare-earth disilicate for the first time. The (Yb0.2Tm0.2Lu0.2Sc0.2Er0.2)2Si2O7 with smaller grain size was prepared by one-step pressureless sintering method. Results of thermal conductivity and coefficient of thermal expansion (CTE) reveal that thermal conductivity of (Yb0.2Tm0.2Lu0.2Sc0.2Er0.2)2Si2O7 bulk material is lower than that all existing EBCs and even most TBCs and potential TEBCs material, which is 0.686 W m−1 °C−1 at 1300 °C. Excellent thermophysical properties indicate that designed (Yb0.2Tm0.2Lu0.2Sc0.2Er0.2)2Si2O7 with small grain size can be used as a promising TEBCs material.
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关键词
Ceramic-matrix composites (CMCs),Thermal properties,Thermal analysis,Sintering
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