Direct observation of the Mottness and p–d orbital hybridization in the epitaxial monolayer α-RuCl₃

Zhongjie Wang,Lu Liu,Haoran Zheng, Meng Zhao,Ke Yang,Chunzheng Wang,Fang Yang,Hua Wu,Chunlei Gao

Nanoscale（2022）

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摘要

In this work, we grow and study the strained monolayer α-RuCl3 on graphene by MBE, STM and DFT calculations. The Mottness and the energy-resolved d–p hybridization, which underlie the mechanism of Kitaev physics, are clearly visualized and elaborated.

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Direct observation of the Mottness and p–d orbital hybridization in the epitaxial monolayer α-RuCl3

Direct observation of the Mottness and p–d orbital hybridization in the epitaxial monolayer α-RuCl₃