In operando simultaneous ATR-IR/Raman spectroscopic investigation of the catalytic activity of supported Pt, Ru, and Pd catalysts in H/D exchange reactions between H2 and D2O

Isaline Bonnin,Raphaël Mereau,Karine De Oliveira Vigier,Thierry Tassaing

Molecular Catalysis（2023）

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摘要

•Catalytic H/D exchange experiments between H2 and D2O catalyzed by supported metals.•The reaction was monitored using in operando simultaneous ATR-IR/Raman spectroscopy.•Pt/Al2O3 had the highest efficiency for H/D exchange, followed by Ru/Al2O3 and Pd/Al2O3.•The enhanced activity of Ru/Al2O3 for glucose hydrogenation is due to active Ru-H species.

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关键词

Isotopic Exchange, Deuterated water, Dihydrogen, Hydrogenation, Glucose, Ruthenium, Platinum, Palladium, In operando spectroscopy

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