Building of sub-monolayer MoS2-x structure to circumvent the scaling relations in N2-to-NH3 electrocatalysis

Wenzhuo Wu,Chunyao Niu,Pengfei Yan,Feng Shi,Chunyan Ma,Xinan Yang,Yu Jia,Jun Chen,Muhammad Ibrar Ahmed,Chuan Zhao,Qun Xu

Applied Catalysis B: Environmental（2021）

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摘要

•A peculiar sub-monolayer MoS2-x structure was synthesized.•The unique sub-monolayer MoS2-x leads to excellent electrochemical NRR performance.•The compressive strain effects were described by AC-STEM and computational simulations.•The circumvention of the scaling relations contributes to the ultralow overpotential.

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关键词

Molybdenum disulphide,Sub-monolayer,Electrocatalysis,Nitrogen reduction reaction,Scaling relation

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