Molecular engineering of donor-acceptor sp2-carbon-linked covalent organic frameworks for enhancing photocatalytic hydrogen production

Min Xu,Shan Shan Yu,Wanru Li,Chuangye Li, Yukai Peng,Fengtao Yu

Polymer Chemistry（2023）

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摘要

Three sp 2 -carbon-linked D–A COFs have been successfully synthesized via a Knoevenagel condensation reaction. The TTh-COF with strong electron-donating unit of benzotrithiophene exhibits an impressive hydrogen evolution rate 22.22 mmol h −1 g −1 .

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关键词

photocatalytic hydrogen production,hydrogen production,molecular engineering,organic frameworks,donor-acceptor,carbon-linked

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