Prediction of stable nanoscale skyrmions in monolayer Fe_5GeTe_2
arxiv(2024)
摘要
Using first-principles calculations and atomistic spin simulations, we
predict stable isolated skyrmions with a diameter below 10 nm in a monolayer of
the two-dimensional van der Waals ferromagnet Fe_5GeTe_2, a material of
significant experimental interest. A very large Dzyaloshinskii-Moriya
interaction (DMI) is observed due to the intrinsic broken inversion symmetry
and strong spin-orbit coupling for monolayer Fe_5GeTe_2. We show that the
nearest-neighbor approximation, often used in literature, fails to describe the
DMI. The strong DMI together with moderate in-plane magnetocrystalline
anisotropy energy allows to stabilize nanoscale skyrmions in out-of-plane
magnetic fields above ≈ 2 T. The energy barriers of skyrmions in
monolayer Fe_5GeTe_2 are comparable to those of state-of-the-art
transition-metal ultra-thin films. We further predict that these nanoscale
skyrmions can be stable for hours at temperatures up to 20 K.
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