Synthetic method of pure-red emissive CsPbI3 under ambient conditions for quantum-dot light-emitting diode application

Kenshin Yoshida,Naoaki Oshita,Taisei Kimura, Mao Goto, Ryosuke Oikawa, Mizuho Uwano,Satoshi Asakura,Takayuki Chiba,Akito Masuhara

APPLIED PHYSICS EXPRESS(2024)

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摘要
Perovskite quantum dots (PeQDs) are expected to be used in ultra-high-definition television (UHDTV) due to their excellent optical properties. However, pure-red emissive (lambda (EL): 620-650 nm) PeQD-based LEDs (PeLEDs) are required for UHDTV with single-halogen PeQDs synthesized under ambient conditions, which is important for practical use. Hence, we established a novel synthetic method to prepare PeQDs under ambient conditions via a different reaction from conventional methods. We successfully prepared PeQDs with pure-red emissivity lambda (PL): 631 nm and near-unity photoluminescence quantum yield. The PeLEDs with the PeQDs showed pure-red emission of 647 nm.
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