The Heisenberg-RIXS instrument at the European XFEL

Justine Schlappa,Giacomo Ghiringhelli,Benjamin E. Van Kuiken,Martin Teichmann,Piter S. Miedema, Jan Torben Delitz, Natalia Gerasimova,Serguei Molodtsov, Luigi Adriano, Bernard Baranasic, Carsten Broers,Robert Carley, Patrick Gessler, Nahid Ghodrati,David Hickin, Le Phuong Hoang,Manuel Izquierdo,Laurent Mercadier,Giuseppe Mercurio,Sergii Parchenko, Marijan Stupar,Zhong Yin,Leonardo Martinelli, Giacomo Merzoni,Ying Ying Peng, Torben Reuss, Sreeju Sreekantan Nair Lalithambika,Simone Techert,Tim Laarmann,Simo Huotari, Christian Schroeter, Burkhard Langer, Tatjana Giessel,Robby Buechner, Jana Buchheim,Vinicius Vaz da Cruz,Sebastian Eckert,Grzegorz Gwalt, Chun-Yu Liu,Frank Siewert, Christian Sohrt,Christian Weniger,Annette Pietzsch,Stefan Neppl, Friedmar Senf,Andreas Scherz,Alexander Föhlisch

arxiv(2024)

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摘要
Resonant Inelastic X-ray Scattering (RIXS) is an ideal X-ray spectroscopy method to push the combination of energy and time resolutions to the Fourier transform ultimate limit, because it is unaffected by the core-hole lifetime energy broadening. And in pump-probe experiments the interaction time is made very short by the same core-hole lifetime. RIXS is very photon hungry so it takes great advantage from high repetition rate pulsed X-ray sources like the European XFEL. The hRIXS instrument is designed for RIXS experiments in the soft X-ray range with energy resolution approaching the Fourier and the Heisenberg limits. It is based on a spherical grating with variable line spacing (VLS) and a position-sensitive 2D detector. Initially, two gratings are installed to adequately cover the whole photon energy range. With optimized spot size on the sample and small pixel detector the energy resolution can be better than 40 meV at any photon energy below 1000 eV. At the SCS instrument of the European XFEL the spectrometer can be easily positioned thanks to air-pads on a high-quality floor, allowing the scattering angle to be continuously adjusted over the 65-145 deg range. It can be coupled to two different sample interaction chamber, one for liquid jets and one for solids, each equipped at the state-of-the-art and compatible for optical laser pumping in collinear geometry. The measured performances, in terms of energy resolution and count rate on the detector, closely match design expectations. hRIXS is open to public users since the summer of 2022.
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