Efficient sunlight-driven dehydrogenative coupling of methane to ethane over a Zn+-modified zeolite

Lü Li,Guo-Dong Li,Chang Yan,Xiao-Yue Mu,Xiao-Liang Pan,Xiao-Xin Zou,Kai-Xue Wang,Jie-Sheng Chen

ANGEWANDTE CHEMIE-INTERNATIONAL EDITION（2011）

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摘要

Sun bath: A Zn+-modified zeolite catalyst showing superior photocatalytic activity for the activation of a C-H bond converted methane into ethane and hydrogen upon irradiation of sunlight (see picture). Light at wavelengths shorter than 390 nm transferred electrons from the zeolite framework to the zinc centers. © 2011 Wiley-VCH Verlag GmbH & Co. KGaA, Weinheim.

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关键词

C-H activation,electron transfer,photocatalysis,zeolites,zinc

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