Greener and efficient epoxidation of 4-vinyl-1-cyclohexene with polystyrene 2-(aminomethyl)pyridine supported Mo(VI) catalyst in batch and continuous reactors

Misbahu Ladan Mohammed,Rene Mbeleck,Dipesh Patel,Debdarsan Niyogi,David C. Sherrington,Basudeb Saha

Chemical Engineering Research and Design（2015）

引用 14|浏览6

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摘要

•Polystyrene 2-(aminomethyl)pyridine supported Mo(VI) complex (i.e. Ps.AMP.Mo) was prepared.•Epoxidation of 4-vinyl-1-cyclohexene with TBHP was catalysed by Ps.AMP.Mo catalyst.•The process is atom efficient and environmentally friendly.•The ANN modelling has successfully predicted the catalytic performance.•Molybdenum leaching from polymer support was due to soluble leached complex.

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关键词

Alkene epoxidation,Artificial neural network (ANN),tert-Butyl hydroperoxide (TBHP),Heterogeneous catalysis,Polymer supported Mo(VI) catalyst,4-Vinyl-1-cyclohexene

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