Reevaluation of neutron flux characterization parameters for NIST RT-2 facility

Journal of Radioanalytical and Nuclear Chemistry(2014)

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摘要
It has been difficult to characterize the thermal to epithermal neutron flux ratio ( f ) and the measure of the nonideal epithermal neutron flux distribution ( α ) for the RT-2 pneumatic rabbit facility at the NIST National Bureau of Standards Reactor (NBSR). In a previous paper, only cadmium-covered irradiations yielded physically reasonable parameters. New measurements were performed using chromium, manganese, cobalt, zinc, zirconium, molybdenum, antimony, gadolinium, lutetium, and gold. The neutron temperature ( T n ) in RT-2 measured using bare lutetium and gold foils gave unphysical values. The bare foil methods for measuring f and α gave inconsistent results. The underlying reasons are demonstrated via MCNP simulation results for cumulative reaction rates of selected isotopes. To determine expected intervals for f , α and T , parametric methods were explored. Measured reaction rate probability per target atom ( R p ) values for the listed elements were fitted to a modified Westcott curve using an iterative least-squares method to verify consistency of measurements and nuclear data. An advanced parametric approach using a detailed MCNP model of the NBSR was used to calculate neutron flux characterization parameters.
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关键词
Neutron activation analysis (NAA),k0 method,Neutron flux characterization,Neutron temperature,Westcott formalism
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