Fabricating Nanogaps between Nanoelectrodes using Dielectrophoresis Technique for Molecular Fluorescence Enhancement

CHINESE JOURNAL OF CHEMICAL PHYSICS(2016)

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摘要
Here we demonstrate the fabrication of nanometer-sized gaps by assembling single coreshell nanoparticles between metallic nanoelectrodes. Protein coated SiO2@Au coreshell nanoparticles are synthesized and positioned between fluorescent molecules-covered electrodes in a controllable way using dielectrophoretic trapping, forming nanogaps sandwiched between nanoparticle and nanoelectrodes. Preliminary photoluminescence measurements show that enhanced molecular fluorescence could be detected from the fluorescent molecules inside the nanogaps. These results pave the way for realizing electrically driven molecular fluorescence based on nanogap electrodes.
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关键词
Nanogap,Nanoelectrode,Dielectrophoresis,Coreshell nanoparticle,Fluorescence enhancement
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