Quantitative theoretical analysis of lifetimes and decay rates relevant in laser cooling BaH

Journal of Quantitative Spectroscopy and Radiative Transfer（2018）

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摘要

•Ab initio lifetimes of the H2Δ, A2Π, B2Σ and E2Π low lying excited states.•Spin-orbit coupling parameters calculated for all states•Electric-dipole decay pathways quantified.•Assessment of laser cooling viability in BaH.

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关键词

BaH isotopologue,Laser cooling,Vibrational and rotational analysis,Molecular parameters,Ab initio quantum chemistry,Spin-orbit coupling

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