C(sp3)–C(sp3) Coupling with a Pd(II) Complex Bearing a Structurally Responsive Ligand

Kyle M. K. Jackman, Benjamin J. Bridge,Ethan R. Sauvé,Christopher N. Rowley,Cameron H. M. Zheng,James M. Stubbs,Paul D. Boyle,Johanna M. Blacquiere

Organometallics（2019）

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摘要

A dimer with two PdII–Me fragments is stabilized by the bridging coordination of the supporting 1-azaallyl/phosphine ligand. Heating the complex results in C(sp3)–C(sp3) bond formation and the release of ethane. Two different palladium products are generated, each with distinct coordination modes of the 1-azaallyl/phosphine ligand.

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