Terahertz Control Of Air Lasing

The coherent emission from ionized nitrogen molecules is of interest for remote sensing and astronomical applications. To initiate the lasing process, we used an intense ultrashort near-infrared (NIR) pulse overlapped with a terahertz (THz) single-cycle pulse. We observed that coherent emission could be seeded and modulated by the amplitude of the THz field, which is the result of a combined effective second-order nonlinear polarization and the nonlinear effects induced by the NIR pump. Our results shed light on the role of intense transient fields in the coherent emission from photoexcited gas molecules.