Ultrafast Ring-Opening Dynamics Of 1,3-Cyclohexadiene Probed Via Time-Resolved High-Harmonic Spectroscopy
2019 CONFERENCE ON LASERS AND ELECTRO-OPTICS (CLEO)（2019）
摘要
We demonstrate the simultaneous observation of the electronic and vibrational dynamics of the photo-isomerizing 1,3-cyclohexadiene via time-resolved high-harmonic spectroscopy. The observed attosecond high-harmonic interference reveals how the excited-state ionization potential evolves along the reaction coordinate. (C) 2019 The Author(s)
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关键词
time-resolved high-harmonic spectroscopy,ultrafast ring-opening dynamics,electronic dynamics,vibrational dynamics,1,3-cyclohexadiene,photo-isomerization,attosecond high-harmonic interference,excited-state ionization potential,reaction coordinate,photoexcitation
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