Promoting Thermodynamically Unfavorable [3,3] Rearrangements by Chemoselective Reduction
Organic letters(2019)
摘要
Herein described is a strategy for promoting thermodynamically unfavorable [3,3] Cope rearrangements. 3,3-Dicyano-1,5-dienes that are resistant to the thermal rearrangement can be promoted under reductive conditions. The reduced Cope products are versatile, bifunctional building blocks.
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