Electronic Structure of $\mathrm{UTe_2}$ Studied by Photoelectron Spectroscopy

arxiv(2019)

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摘要
The electronic structure of the unconventional superconductor $\mathrm{UTe_2}$ was studied by resonant photoelectron spectroscopy (RPES) and angle-resolved photoelectron spectroscopy (ARPES) with soft X-ray synchrotron radiation. The partial $\mathrm{U}~5f$ density of states of $\mathrm{UTe_2}$ were imaged by the $\mathrm{U}~4d$--$5f$ RPES and it was found that the $\mathrm{U}~5f$ state has an itinerant character, but there exists an incoherent peak due to the strong electron correlation effects. Furthermore, an anomalous admixture of the $\mathrm{U}~5f$ states into the $\mathrm{Te}~5p$ bands was observed at a higher binding energy, which cannot be explained by band structure calculations. On the other hand, the band structure of $\mathrm{UTe_2}$ was obtained by ARPES and its overall band structure were mostly explained by band structure calculations. These results suggest that the $\mathrm{U}~5f$ states of $\mathrm{UTe_2}$ have itinerant but strongly-correlated nature with enhanced hybridization with the $\mathrm{Te}~5p$ states.
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