Corrigendum for “Solar-light-active silver phosphate/titanium dioxide/silica heterostructures for photocatalytic removal of organic dye” [J. Clean. Prod. 254 (2020) 120031]

Journal of Cleaner Production(2021)

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摘要
A synergistic combination of surface adsorption capabilities and photocatalytic efficiency is crucial for the removal of pollutants from water. Here, the efficacy of such a process is explored through the assembly of a heterostructured photocatalyst (Ag3PO4/TiO2/SiO2) by loading silver phosphate (Ag3PO4) onto titanium dioxide (TiO2: P25)-coated silica (SiO2) felt. This heterostructure demonstrated an enhanced tendency to absorb light due to its significantly low band-gap energy of 2.5 eV. As such, it exhibited enhanced photocatalytic performance to efficiently degrade an organic dye (methylene blue) under solar-light irradiation (e.g., 30% and 10% relative to pristine P25 and P25-coated SiO2 felt, respectively). The maximum degradation efficiency for methylene blue was 99% with a first-order kinetic model (k = 0.39 min−1). The calculated quantum yield of Ag3PO4/TiO2/SiO2 (3.26 × 10−3 molecules/photon) was significantly higher than that of other photocatalytic systems (e.g., ∼3260 times other reported hetrostructures, e.g., rGO/TiO2, Ni-doped/TiO2, and Cds/CoFe2O4) with good reusability in terms of the degradation efficiency (e.g., 99% for the first cycle and 81% for the fourth). Ag3PO4/TiO2/SiO2 is therefore recommended for the efficient treatment of organic pollutants in wastewater systems.
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关键词
Heterojunction,Photocatalyst,Silver phosphate,Titanium dioxide,Organic dye,Silica felt
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