Simulation Of Photo-Electron Spectrum And Electron Scattering By Dual Time Propagation

A dual time propagation approach is introduced to describe electron scattering and ionization. The space is divided into two regions, a central region with a full time-dependent Hamiltonian and an outer region where the kinetic operator and the laser field dominate. The two regions are connected by a source term. Time-dependent density functional theory calculations of wave packet scattering on molecules and photoelectron spectrum due to circularly polarized laser are presented to illustrate the efficiency and applicability of the approach.