Computational Device Optimization And Parameter Extraction For Perovskite-Based Solar Cells

We present a comprehensive approach to the characterization and modeling of photovoltaic metal-halide perovskite single junction devices and perovskite-silicon tandem solar cells. The framework is based on 1D opto-electronic device simulation in steady-state and transient modes as well as frequency domain including specific features of the perovskite materials such as mobile ions, combined with a broad variety of device characterization experiments. As a salient feature, advanced optimization algorithms are used for reliable parameter extraction and opto-electronic device optimization purposes in both single junction and tandem solar cell architectures.