Molecular High-Order Harmonic Generation By Counter-Rotating Elliptically Polarized Intense Pulses

We present a scheme to produce the selected left or right elliptically polarized high-order harmonic generation. By adopting bichromatic counter-rotating colinear elliptically polarized pulses, their interaction with oxygen molecule are calculated under the framework of time-dependent density functional theory. Here we show that the helicity-selective high harmonics with tunable ellipticity are generated by changing the ellipticity of one of the pump pulses. Because of the interference of the degenerate highest occupied molecular orbitals, tunable ellipticity in a wide spectral range is obtained. This scheme can be used to synthesize attosecond pulses with controlled ellipticity and helicity.