Nanocarbon Materials-Based Solar Cells
MATERIALS FOR SUSTAINABLE ENERGY STORAGE AT THE NANOSCALE(2023)
摘要
In this presentation, we introduce our recent research progress on organic and perovskite solar cells using functionalized nanocarbon materials. We applied wet-processed scalable single-walled carbon nanotubes (SWCNT) films to transparent and back electrodes in organic solar cells for large area solar cells. Gas-phase growth SWCNT was dispersed with sodium dodecylbenzenesulfonate surfactant in an organic solvent and solution-coated on a treated glass substrate to make a SWCNT film as a transparent electrode. We achieved the first high efficiency e-DIPS/wet-processed SWCNT film electrode in organic solar cells with a best-efficiency of 5.93% through the optimized HNO3 doping methodology. We also report enhanced hole-transporting ability of widely utilized poly(3,4-ethylenedioxythiophene)-poly(styrenesulfonate) (PEDOT:PSS) achieved by applying cationic nitrogen-doped graphene (CNG) as a p-type modifier for efficient organic solar cells. The power conversion efficiency of the CNG-coated PEDOT:PSS-applied OSC reaches 2.76% using poly(3-hexylthiophene), which is an increase of 40% compared to that of the pristine PEDOT:PSS-applied OSC (1.96%). This technology improved the efficiency of organic solar cells using a low-bandgap polymer from 6.54% to 7.79%. The significantly enhanced performance is contributed by the increased hole-transporting ability, and the improved interfacial morphology of PEDOT:PSS.
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