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Ultrafast Optically-Induced Melting of Trimer Clusters in 1T’-Tate2

K. M. Siddiqui,D. B. Durham,F. Cropp,S. Rajpurohit,C. Ophus,Y. Zhu, J. D. Carlström, C. Stavrakas, Z. Mao, A. Raja, P. Musumeci, L. Z. Tan, A. M. Minor, D. Filippetto, R. A. Kaindl

Frontiers in Optics + Laser Science 2021(2021)

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摘要
Relativistic ultrafast electron diffraction is used to track the transient structural dynamics of tantalum ditelluride. We observe rapid photo-induced melting of its low-temperature trimer superstructure as driven by intra-trimer charge transfer.
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