Anisotropy-driven quantum criticality in an intermediate valence system

NATURE COMMUNICATIONS(2022)

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摘要
Intermetallic compounds containing f -electron elements have been prototypical materials for investigating strong electron correlations and quantum criticality (QC). Their heavy fermion ground state evoked by the magnetic f -electrons is susceptible to the onset of quantum phases, such as magnetism or superconductivity, due to the enhanced effective mass ( m * ) and a corresponding decrease of the Fermi temperature. However, the presence of f -electron valence fluctuations to a non-magnetic state is regarded an anathema to QC, as it usually generates a paramagnetic Fermi-liquid state with quasiparticles of moderate m * . Such systems are typically isotropic, with a characteristic energy scale T 0 of the order of hundreds of kelvins that require large magnetic fields or pressures to promote a valence or magnetic instability. Here we show the discovery of a quantum critical behaviour and a Lifshitz transition under low magnetic field in an intermediate valence compound α -YbAlB 4 . The QC origin is attributed to the anisotropic hybridization between the conduction and localized f -electrons. These findings suggest a new route to bypass the large valence energy scale in developing the QC.
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Electronic properties and materials,Magnetic properties and materials,Phase transitions and critical phenomena,Science,Humanities and Social Sciences,multidisciplinary
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