Na_2.4Al_0.4Mn_2.6O₇ anionic redox cathode material for sodium-ion batteries – a combined experimental and theoretical approach to elucidate its charge storage mechanism

Cindy Soares,Begoña Silván,Yong-Seok Choi,Veronica Celorrio,Valerie R. Seymour,Giannantonio Cibin,John M. Griffin,David O. Scanlon,Nuria Tapia-Ruiz

Journal of Materials Chemistry A（2022）

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摘要

Al substitution and subsequent Na excess in Na2Mn3O7 were achieved by a ceramic method, realizing the high-performance Na2.4Al0.4Mn2.6O7 oxygen-redox cathode for Na-ion batteries. A comparison between the two cathodes revealed the role of Al doping.

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Na2.4Al0.4Mn2.6O7 anionic redox cathode material for sodium-ion batteries – a combined experimental and theoretical approach to elucidate its charge storage mechanism

Na_2.4Al_0.4Mn_2.6O₇ anionic redox cathode material for sodium-ion batteries – a combined experimental and theoretical approach to elucidate its charge storage mechanism