An anhydrous precursor approach to BaYF5-based upconverting nanocrystals
JOURNAL OF THE INDIAN CHEMICAL SOCIETY(2022)
摘要
With an objective to have easy access to high quality BaYF5 matrix, we report here new anhydrous precursors of barium and yttrium which show a good compatibility in terms of co-thermal decomposition. These complexes not only fill the void of precursors for Ba-based upconverting (UC) nanomaterials but also provide a way to minimize the -OH concentration around these nanocrystals (NCs) to enhance their UC efficiency without requiring the usual core-shell structure. The precursors and the BaYF5 NCs co-doped with Yb3+/Tm3+ ions were thoroughly characterized. The NCs were studied for upconversion properties and preliminary results are presented here. On the basis of these results, a mechanism for the energy transfer in Yb-Tm system is proposed.
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关键词
Molecular precursor, Trifluoroacetate, Hot -injection, Anhydrous synthesis, BaYF 5, Upconversion
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