Novel pyrazole-based carboxylate ligand as a building block for assembling lanthanides in luminescent 2D and 3D MOFs

Alexey M. Lunev, Anastasia V. Sidoruk,Victoria E. Gontcharenko, Mikhail A. Kiskin,Ilya V. Taydakov,Yury A. Belousov,Andrey A. Drozdov

Inorganica Chimica Acta（2022）

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摘要

•New pyrazole-based carboxylic ligand 1-(carboxymethyl)-1H-pyrazole-3,5-dicarboxylic acid (H3L) has been prepared.•Two new families of lanthanide complexes [LnL(H2O)2]n, Ln = La-Tb and [LnL(H2O)]n, Ln = Dy-Lu has been prepared and studied.•It was shown that the ligand H3L is able to sensitize the lanthanide luminescence emitting in VIS-region, especially Tb3+.

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关键词

Lanthanides,Luminescence,Carboxylates,Pyrazoles,Europium,Terbium,Gadolinium,Samarium,Dysprosium,Crystal structure

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