Two-dimensional ferromagnetic extension of a topological insulator

P. Kagerer,C. I. Fornari, S. Buchberger, T. Tschirner,L. Veyrat,M. Kamp,A. V. Tcakaev,V. Zabolotnyy,S. L. Morelhão, B. Geldiyev, S. Müller, A. Fedorov, E. Rienks, P. Gargiani,M. Valvidares, L. C. Folkers,A. Isaeva,B. Büchner, V. Hinkov,R. Claessen,H. Bentmann, F. Reinert

arXiv (Cornell University)(2022)

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摘要
Inducing a magnetic gap at the Dirac point of the topological surface state (TSS) in a 3D topological insulator (TI) is a route to dissipationless charge and spin currents. Ideally, magnetic order is present only at the surface and not in the bulk, e.g. through proximity of a ferromagnetic (FM) layer. However, such a proximity-induced Dirac mass gap has not been observed, likely due to insufficient overlap of TSS and the FM subsystem. Here, we take a different approach, namely FM extension, using a thin film of the 3D TI Bi$_2$Te$_3$, interfaced with a monolayer of the lattice-matched van der Waals ferromagnet MnBi$_2$Te$_4$. Robust 2D ferromagnetism with out-of-plane anisotropy and a critical temperature of $\text{T}_\text{c}\approx$~15 K is demonstrated by X-ray magnetic dichroism and electrical transport measurements. Using angle-resolved photoelectron spectroscopy, we observe the opening of a sizable magnetic gap in the 2D FM phase, while the surface remains gapless in the paramagnetic phase above T$_c$. This sizable gap indicates a relocation of the TSS to the FM ordered Mn moments near the surface, which leads to a large mutual overlap.
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