Intelligent Safeguarding Leather with Excellent Energy Absorption Via the Toughness-Flexibility Coupling Designation

High-performance intelligent body armors with both soft wearability and good energy absorption are increas-ingly required in modern social life. Leather, a breathable, pliable, and tough natural material has extensive applications in the anti-impact field. In this study, a multifunctional Leather/CNT-SSG/PU sandwich structure with high energy absorption and excellent sensing monitoring properties is designed by integrating tough leather and flexible conductive shear stiffening gel (CNT-SSG). The maximum force dissipation capacity of the Leather/ CNT-SSG/PU reaches 84 % in the drop hammer test and the limit penetration velocity up to 142.4 m/s in the ballistic test. Moreover, the Leather/CNT-SSG/PU exhibits excellent stress wave dissipation properties due to the hierarchical structure. By introducing the interdigital electrode array on the non-woven fabric layer, a bullet-proof vest (Leather/CNT-SSG/NWF) with intelligent anti-impact performance and in situ monitoring behavior is successfully achieved. This toughness and flexibility coupling designation provides a novel method for next -generation soft body armor.