The emergence of drop-type and thin-layer-type quasi-liquid layers on ice crystal surfaces and their thermodynamic origin

Journal of Crystal Growth(2022)

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摘要
•Two kinds of quasi-liquid layers (QLLs) with different morphologies (droplets and thin layers) are observed in-situ on basal and prism faces of ice crystals by laser confocal microscopy combined with differential interference contrast microscopy (LCM-DIM).•The drop-type and thin-layer-type QLLs are 20- and 200-times less fluidic than bulk water, respectively.•The drop-type and thin-layer-type morphologies are formed by the wetting transition of QLLs on ice crystal surfaces.•The drop-type and thin-layer-type QLLs are a metastable phase that is formed kinetically only in supersaturated or undersaturated water vapor.
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关键词
A1. Surface melting,A1. Quasi-liquid layer,A1. Optical microscopy,A2. Growth from vapor,B1. Ice
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