A diamantane-4,9-dicarboxylate based UiO-66 analogue: challenging larger hydrocarbon cage platforms

Vasily Gvilava, Maximilian Vieten,Robert Oestreich,Dennis Woschko, Moritz Steinert,Ishtvan Boldog,Roman Bulanek,Natalie A. Fokina,Peter R. Schreiner,Christoph Janiak

CRYSTENGCOMM（2022）

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摘要

The first use of a bulky barrel-shaped ligand is demonstrated in HHUD-3, with accessible porosity only feasible for a defect structure. With 35%+ missing linker defects and S-BET = 890 m(2)g(-1) (N-2), HHUD-3 features higher CH4 but lower CO2 and H-2 adsorption than UiO-66.

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