Measurement of 134 Xe(n,2n) 133m,g Xe reaction cross sections in 14-MeV region with detailed uncertainty quantification

Nuclear Science and Techniques(2023)

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摘要
A lead-shielded HPGe detector and offline γ-ray spectra of the residual product were used to measure the cross section (CS) and ratios of isomeric CS (σ m /σ g ) in 134 Xe(n,2n) 133m,g Xe reactions at different energies (13.5 MeV, 13.8 MeV, 14.1 MeV, 14.4 MeV, 14.8 MeV) relative to the 93 Nb(n,2n) 92m Nb reaction CS. The target was high-purity natural Xe gas under high pressure. The T(d,n) 4 He reaction produces neutrons. TALYS code (version 1.95) for nuclear reactions was used for calculations, with default parameters and nuclear level density models. The uncertainties in the measured CS data were thoroughly analyzed using the covariance analysis method. The results were compared with theoretical values, evaluation data, and previous experimental findings. CS data of the 134 Xe(n,2n) 133m Xe and 134 Xe(n,2n) 133g Xe reactions and the corresponding isomeric CS ratios at 13.5 MeV, 13.8 MeV, and 14.1 MeV neutron energies are reported for the first time. This research advances our knowledge of pre-equilibrium emission in the (n,2n) reaction channel by resolving inconsistencies in the Xe data.
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关键词
134Xe(n,2n) reactions,14-MeV neutrons,Cross sections (CSs),Isomeric ratios (IRs),Covariance analysis
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